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• W2783001208 abstract "We demonstrate that the population of the molecular rotational state through a stimulated impulsive Raman excitation can be controlled by tailoring the femtosecond laser pulse with a V-style phase modulation. The results show that, by precisely manipulating the modulation parameters, both the odd and even populations of the molecular rotational state can be completely suppressed or reconstructed. Meanwhile, the relative excitation between the odd and even populations can be obtained. Finally, we show that field-free molecular alignment can be controlled due to the modulation of the molecular rotational state populations." @default.
• W2783001208 created "2018-01-26" @default.
• W2783001208 creator A5036938499 @default.
• W2783001208 creator A5053505923 @default.
• W2783001208 date "2018-01-01" @default.
• W2783001208 modified "2023-10-06" @default.
• W2783001208 title "Controlling population of the molecular rotational state and the alignment theoretically by tailored femtosecond laser pulse" @default.
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• W2783001208 doi "https://doi.org/10.1098/rsos.171502" @default.
• W2783001208 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5792930" @default.
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