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- W2783008783 abstract "N-doped TiO2 (NT) was proven to be efficient for monuron decay via peroxymonosulfate (PMS) activation under visible LED (Vis LED). The activation mechanism revealed that OH and SO4− have a critical role in the monuron decay with a ratio of about 3 to 1, respectively; and the holes at the catalyst surface are the main precursors in forming SO4−. The NT/PMS/Vis LED hybrid process was found to be an effective approach under a wide solution pH range of 2.5–9.2 (>80% decay). Interestingly, the highest efficiency was observed at pH 9.2 due to the contribution of PMS/Vis LED process by generating both OH and SO4− at alkaline pH. However, the decay rate of monuron was inhibited at pH 11.6 due to the dissociation of OH into O− and the electrostatic repulsion among reagents. The process was also suitable for ion-rich wastewater since no significant reduction in the performance was induced in the presence of high concentrations of inorganic anions. Furthermore, the process was proven to be a promising approach for mineralization of monuron and its intermediates. Twenty reaction intermediates were detected and five of them are newly reported. A novel mathematical model was established based on reaction intermediates using a parallel-serial-irreversible reaction approach, which is helpful in predicting the detoxification extent of hazardous intermediates." @default.
- W2783008783 created "2018-01-26" @default.
- W2783008783 creator A5020645897 @default.
- W2783008783 creator A5056008057 @default.
- W2783008783 date "2018-04-01" @default.
- W2783008783 modified "2023-10-05" @default.
- W2783008783 title "Monuron photodegradation using peroxymonosulfate activated by non-metal-doped TiO2 under visible LED and the modeling via a parallel-serial kinetic approach" @default.
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- W2783008783 doi "https://doi.org/10.1016/j.cej.2018.01.036" @default.
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