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• W2783103484 abstract "A low-temperature ammonia synthesis process is required for on-site synthesis. Barium-doped calcium amide (Ba-Ca(NH2 )2 ) enhances the efficacy of ammonia synthesis mediated by Ru and Co by 2 orders of magnitude more than that of a conventional Ru catalyst at temperatures below 300 °C. Furthermore, the presented catalysts are superior to the wüstite-based Fe catalyst, which is known as a highly active industrial catalyst at low temperatures and pressures. Nanosized Ru-Ba core-shell structures are self-organized on the Ba-Ca(NH2 )2 support during H2 pretreatment, and the support material is simultaneously converted into a mesoporous structure with a high surface area (>100 m2 g-1 ). These self-organized nanostructures account for the high catalytic performance in low-temperature ammonia synthesis." @default.
• W2783103484 created "2018-01-26" @default.
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• W2783103484 date "2018-02-02" @default.
• W2783103484 modified "2023-10-17" @default.
• W2783103484 title "Self-organized Ruthenium-Barium Core-Shell Nanoparticles on a Mesoporous Calcium Amide Matrix for Efficient Low-Temperature Ammonia Synthesis" @default.
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• W2783103484 doi "https://doi.org/10.1002/anie.201712398" @default.
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• W2783103484 hasPublicationYear "2018" @default.
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