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- W2783137249 endingPage "1459" @default.
- W2783137249 startingPage "1410" @default.
- W2783137249 abstract "The borrowing hydrogen (BH) principle, also called hydrogen auto-transfer, is a powerful approach which combines transfer hydrogenation (avoiding the direct use of molecular hydrogen) with one or more intermediate reactions to synthesize more complex molecules without the need for tedious separation or isolation processes. The strategy which usually relies on three steps, (i) dehydrogenation, (ii) intermediate reaction, and (iii) hydrogenation, is an excellent and well-recognized process from the synthetic, economic, and environmental point of view. In this context, the objective of the present review is to give a global overview on the topic starting from those contributions published prior to the emergence of the BH concept to the most recent and current research under the term of BH catalysis. Two main subareas of the topic (homogeneous and heterogeneous catalysis) have been identified, from which three subheadings based on the source of the electrophile (alkanes, alcohols, and amines) have been considered. Then the type of bond being formed (carbon-carbon and carbon heteroatom) has been taken into account to end-up with the intermediate reaction working in tandem with the metal-catalyzed hydrogenation/dehydrogenation step. The review has been completed with the more recent advances in asymmetric catalysis using the BH strategy." @default.
- W2783137249 created "2018-01-26" @default.
- W2783137249 creator A5000454699 @default.
- W2783137249 creator A5024351567 @default.
- W2783137249 creator A5030798322 @default.
- W2783137249 date "2018-01-10" @default.
- W2783137249 modified "2023-10-17" @default.
- W2783137249 title "Advances in One-Pot Synthesis through Borrowing Hydrogen Catalysis" @default.
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