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- W2783194365 abstract "Amino acid based diamides are widely used as a substructure in supramolecular polymers and are also key components of polypeptides that help to understand protein folding. The interplay of folding and aggregation of a diamide was used to achieve seed-initiated supramolecular polymerization. For that purpose, a pyrene-substituted diamide was synthesized in which pyrene is used as a tracer to monitor the supramolecular polymerization. Thermodynamics and time-dependent studies revealed that the folding of the diamide moiety, via the formation of intramolecular hydrogen bonds, effectively prevents a spontaneous nucleation that leads to supramolecular polymerization. Under such out-of-equilibrium conditions, the addition of seeds successfully initiates the supramolecular polymerization. These results demonstrate the utility of such amino acid based diamides in programmable supramolecular polymerizations." @default.
- W2783194365 created "2018-01-26" @default.
- W2783194365 creator A5013623476 @default.
- W2783194365 creator A5015471677 @default.
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- W2783194365 date "2018-02-02" @default.
- W2783194365 modified "2023-10-03" @default.
- W2783194365 title "Seeded Polymerization through the Interplay of Folding and Aggregation of an Amino-Acid-based Diamide" @default.
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- W2783194365 doi "https://doi.org/10.1002/anie.201712119" @default.
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