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• W2783197013 abstract "Plasmonic waveguides can greatly enhance nonlinear light–matter interactions through strong field confinement. However, achieving high performance nonlinear plasmonic devices remains challenging because of optical losses and material damage. Here we investigate the ultimate Kerr nonlinear performance of plasmonic waveguides. We account for optical damage by requiring that the local electric field intensity does not exceed the damage threshold of the nonlinear material. This allows us to factorize the fundamental limitations into those stemming from the constituent materials’ linear and nonlinear properties, and from the mode characteristics. We define quality coefficients for the metal and for the nonlinear dielectric so that these materials can be selected appropriately, and illustrate their utility by application to surface plasmon polaritons (SPPs). We further propose the concept of nonlinear effectiveness in order to quantify a mode’s ability to exploit the material’s nonlinearity. We find that the full exploitation of the material’s maximum nonlinearity requires a uniform field in addition to slow light effects. This is exemplified by the discovery that the maximum nonlinearity of Metal–Dielectric–Metal structures can be stronger than that of the bulk material. These counterintuitive insights provide deep understanding into the ultimate performance of nonlinear waveguides, and point to novel approaches to achieve practical, high performance nonlinear plasmonic devices." @default.
• W2783197013 created "2018-01-26" @default.
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• W2783197013 date "2018-01-12" @default.
• W2783197013 modified "2023-10-02" @default.
• W2783197013 title "Fundamental Limitations to the Ultimate Kerr Nonlinear Performance of Plasmonic Waveguides" @default.
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• W2783197013 doi "https://doi.org/10.1021/acsphotonics.7b01331" @default.
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