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- W2783256954 abstract "A palladium-catalyzed asymmetric intramolecular allylic C-H amination controlled by a chiral phosphoramidite ligand was established for the preparation of various substituted chiral hydropyrimidinones, the precursors of hydropyrimidines, in high yields with high enantioselectivities. In particular, dienyl sodium N-sulfonyl amides bearing an arylethene-1-sulfonyl group underwent a sequential allylic C-H amination and intramolecular Diels-Alder (IMDA) reaction to produce chiral fused tricyclic tetrahydropyrimidinone frameworks in high yields and with high levels of stereoselectivity. Significantly, this method was used as the key step in an asymmetric synthesis of letermovir." @default.
- W2783256954 created "2018-01-26" @default.
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- W2783256954 creator A5080902320 @default.
- W2783256954 creator A5082627703 @default.
- W2783256954 date "2017-11-15" @default.
- W2783256954 modified "2023-10-03" @default.
- W2783256954 title "Access to Chiral Hydropyrimidines through Palladium-Catalyzed Asymmetric Allylic C−H Amination" @default.
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- W2783256954 doi "https://doi.org/10.1002/anie.201709681" @default.
- W2783256954 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29063650" @default.
- W2783256954 hasPublicationYear "2017" @default.
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