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• W2783282960 abstract "The development of new nonlinear optical (NLO) materials for deep-ultraviolet (DUV) applications is in great demand. However, the synthesis of an ideal DUV NLO crystal is a serious challenge. Herein, three new alkali-metal fluorooxoborates, AB4O6F (A=K, Rb, and Cs, and a mixed cation between two of them), were successfully synthesized by cation regulation. It is found that all reported compounds exhibit short UV absorption edges (<190 nm), and show second harmonic generation (SHG) responses ranging from 0.8 to 1.9 KH2PO4 (KDP). Interestingly, by judicious selection of the A-site alkali-metal cations, the arrangement of NLO-active structural units is fine-tuned to an optimal configuration, which contributes to large SHG responses." @default.
• W2783282960 created "2018-01-26" @default.
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• W2783282960 date "2018-01-18" @default.
• W2783282960 modified "2023-10-16" @default.
• W2783282960 title "Cation-Tuned Synthesis of Fluorooxoborates: Towards Optimal Deep-Ultraviolet Nonlinear Optical Materials" @default.
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• W2783282960 doi "https://doi.org/10.1002/ange.201712168" @default.
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• W2783282960 hasPublicationYear "2018" @default.
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