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- W2783295596 abstract "Li2MnO3-based Li-rich cathode materials can offer high capacities for lithium-ion batteries but suffer from poor rate capability, low initial coulombic efficiency, and voltage fade upon extended cycling. Significant attention has been focused on the replacement of Li2MnO3 with other materials featuring Li2MO3 (M = Ru, Mo, etc.) components; however, the cycle performance of these materials is inferior. Herein, coating with Al2O3 is proposed to improve the electrochemical performance of the Li2RuO3-based Li-rich cathode material Li1.2Ni0.2Mn0.2Ru0.4O2. Rietveld refinement data indicate Ru-Ru dimer formation in these samples. The Al2O3 coating can enhance the initial coulombic efficiency, cycling stability, rate performance, and mitigate the voltage decay. In situ X-ray diffraction (XRD) demonstrates that the compound remains a layered structure during the first cycle. The formation of Ru-Ru dimers is suggested to be responsible for the unusual lattice parameter changes during the initial charge." @default.
- W2783295596 created "2018-01-26" @default.
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- W2783295596 date "2018-04-01" @default.
- W2783295596 modified "2023-10-13" @default.
- W2783295596 title "Al2O3 coated Li1.2Ni0.2Mn0.2Ru0.4O2 as cathode material for Li-ion batteries" @default.
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- W2783295596 doi "https://doi.org/10.1016/j.jallcom.2018.01.146" @default.
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