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- W2783479107 abstract "A direct catalytic Mannich-type reaction of α-oxygen-functionalized amides was achieved. The use of 7-azaindoline amide was crucial to facilitate direct enolization and subsequent stereoselective addition to imines in a cooperative catalytic system comprising a soft Lewis acid and Brønsted base. The operationally simple room-temperature protocol furnished a syn-Mannich adduct with high stereoselectivity. Divergent functional group transformation of the amide moiety of the product allowed for expeditious access to enantioenriched syn-configured α-hydroxy-β-amino carboxylic acid derivatives, highlighting the synthetic utility of the present catalysis." @default.
- W2783479107 created "2018-01-26" @default.
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- W2783479107 date "2018-01-14" @default.
- W2783479107 modified "2023-10-17" @default.
- W2783479107 title "Direct Catalytic Asymmetric Mannich-Type Reaction en Route to α-Hydroxy-β-amino Acid Derivatives" @default.
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- W2783479107 doi "https://doi.org/10.1021/acs.orglett.7b03609" @default.
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