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- W2783808958 abstract "Gold(I) complexes bearing sterically demanding phosphine ligands such as tBuXphos catalyze the cascade Rautenstrauch rearrangement/[4 + 3] cycloaddition of 1-ethynyl-2-propenyl esters. The reaction provides an efficient and straightforward route to bicyclo[3.2.1]octa-3,6-dienes with high regio- and stereoselectivity. The formation of the [4 + 3] cycloadducts likely proceeds through the cycloaddition of a gold(I) carbenoid/gold-stabilized allyl cation intermediate with cyclopentadiene arising from Rautenstrauch rearrangement." @default.
- W2783808958 created "2018-01-26" @default.
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- W2783808958 date "2018-01-22" @default.
- W2783808958 modified "2023-10-17" @default.
- W2783808958 title "Ligand-Effect in Gold(I)-Catalyzed Rautenstrauch Rearrangement: Regio- and Stereoselective Synthesis of Bicyclo[3.2.1]octa-3,6-dienes through Cyclodimerization of 1-Ethynyl-2-propenyl Esters" @default.
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- W2783808958 doi "https://doi.org/10.1021/acs.joc.7b02816" @default.
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