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- W2783865646 abstract "We report here a new methodology for the formation of freestanding nanotubes composed of individual gold nanoparticles (NPs) cross-linked by coordination complexes or porphyrin molecules using WS2 nanotubes (INT-WS2) as a template. Our method consists of three steps: (i) coverage of these robust inorganic materials with monodispersed and dense monolayers of gold NPs, (ii) formation of a molecular AuNP network by exposing these decorated tubes to solutions containing a ruthenium polypyridyl complex or meso-tetra(4-pyridyl)porphyrin, and (iii) removal of the INT-WS2 template with a hydrogen peroxide solution. Nanoindentation of the template-free AuNP tubes with atomic force microscopy indicates a radial elastic modulus of 4 GPa. The template-free molecular AuNP tubes are characterized using scanning and transmission electron microscopy, energy-dispersive X-ray spectroscopy, and micro-Raman spectroscopy. The methodology provides a convenient and scalable strategy for the realization of molecular AuNP tubes with a defined length and diameter, depending on the dimensions of the template." @default.
- W2783865646 created "2018-01-26" @default.
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- W2783865646 date "2018-02-06" @default.
- W2783865646 modified "2023-09-26" @default.
- W2783865646 title "Tubular Hybrids: A Nanoparticle—Molecular Network" @default.
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- W2783865646 doi "https://doi.org/10.1021/acs.langmuir.7b03125" @default.
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