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• W2784094443 abstract "The generally accepted three-step mechanism of propene oxidation to acrolein includes abstraction of two hydrogen atoms and addition of one oxygen atom. The first step is a well-known H-abstraction from the methyl group. The sequence of two other steps is unclear. We investigated the reaction in quasi-catalytic mode at 100–200 °C with extraction and analysis of accumulated surface products. The reaction intermediate, surface ether of allyl alcohol, was identified. This strongly proves that O-addition precedes the second H-abstraction. Activation energy and kinetic isotope effect of the quasi-catalytic reaction correlate with appropriate parameters of the conventional catalytic process." @default.
• W2784094443 created "2018-01-26" @default.
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• W2784094443 date "2018-01-16" @default.
• W2784094443 modified "2023-09-26" @default.
• W2784094443 title "Quasi-Catalytic Identification of Intermediates in the Oxidation of Propene to Acrolein over a Multicomponent Bi–Mo Catalyst" @default.
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• W2784094443 doi "https://doi.org/10.1021/acscatal.7b03833" @default.
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