Matches in SemOpenAlex for { <https://semopenalex.org/work/W2785171078> ?p ?o ?g. }
Showing items 1 to 73 of
73
with 100 items per page.
- W2785171078 abstract "The importance of fast vibrations in enhancing and controlling energy transfer and conversion in biomolecules is an issue of current debate. In this article we show that coupling between localised high-frequency vibrations and electronic degrees of freedom is fundamental for efficient excitation transport in photosynthetic light-harvesting systems with high degree of disorder. We consider the cryptophyte antennae protein phycoerythrin 545 and discuss how the balance between electronic interactions and coupling to fast vibronic modes supports the biological function of these antennae by generating a non-cascaded transport that leads to a rapid, directed and wider spatial distribution of excitation energy across the complex. Furthermore, we illustrate signatures of vibronic influence in the beating of excitonic coherences and show that mechanisms supporting coherent evolution of excitons also assist coupling to selected modes that enhance energy transfer to preferential sites in the complex. We therefore argue that, in the presence of strong coupling between highly localised electronic excitations and quantised vibrations, a concrete and important function for quantum coherent dynamics is to optimise resonances that promote fast and effective energy distribution." @default.
- W2785171078 created "2018-02-02" @default.
- W2785171078 creator A5029838157 @default.
- W2785171078 creator A5038050336 @default.
- W2785171078 creator A5056017337 @default.
- W2785171078 creator A5076241774 @default.
- W2785171078 date "2012-03-20" @default.
- W2785171078 modified "2023-09-27" @default.
- W2785171078 title "The fundamental role of localised vibrations in excitation dynamics in photosynthetic light-harvesting systems" @default.
- W2785171078 hasPublicationYear "2012" @default.
- W2785171078 type Work @default.
- W2785171078 sameAs 2785171078 @default.
- W2785171078 citedByCount "0" @default.
- W2785171078 crossrefType "posted-content" @default.
- W2785171078 hasAuthorship W2785171078A5029838157 @default.
- W2785171078 hasAuthorship W2785171078A5038050336 @default.
- W2785171078 hasAuthorship W2785171078A5056017337 @default.
- W2785171078 hasAuthorship W2785171078A5076241774 @default.
- W2785171078 hasConcept C106447425 @default.
- W2785171078 hasConcept C121332964 @default.
- W2785171078 hasConcept C131584629 @default.
- W2785171078 hasConcept C159467904 @default.
- W2785171078 hasConcept C171250308 @default.
- W2785171078 hasConcept C17729963 @default.
- W2785171078 hasConcept C191897082 @default.
- W2785171078 hasConcept C192562407 @default.
- W2785171078 hasConcept C198394728 @default.
- W2785171078 hasConcept C208081375 @default.
- W2785171078 hasConcept C49853544 @default.
- W2785171078 hasConcept C62520636 @default.
- W2785171078 hasConcept C83581075 @default.
- W2785171078 hasConcept C84114770 @default.
- W2785171078 hasConceptScore W2785171078C106447425 @default.
- W2785171078 hasConceptScore W2785171078C121332964 @default.
- W2785171078 hasConceptScore W2785171078C131584629 @default.
- W2785171078 hasConceptScore W2785171078C159467904 @default.
- W2785171078 hasConceptScore W2785171078C171250308 @default.
- W2785171078 hasConceptScore W2785171078C17729963 @default.
- W2785171078 hasConceptScore W2785171078C191897082 @default.
- W2785171078 hasConceptScore W2785171078C192562407 @default.
- W2785171078 hasConceptScore W2785171078C198394728 @default.
- W2785171078 hasConceptScore W2785171078C208081375 @default.
- W2785171078 hasConceptScore W2785171078C49853544 @default.
- W2785171078 hasConceptScore W2785171078C62520636 @default.
- W2785171078 hasConceptScore W2785171078C83581075 @default.
- W2785171078 hasConceptScore W2785171078C84114770 @default.
- W2785171078 hasLocation W27851710781 @default.
- W2785171078 hasOpenAccess W2785171078 @default.
- W2785171078 hasPrimaryLocation W27851710781 @default.
- W2785171078 hasRelatedWork W1494757885 @default.
- W2785171078 hasRelatedWork W1647669928 @default.
- W2785171078 hasRelatedWork W1991695217 @default.
- W2785171078 hasRelatedWork W2024542242 @default.
- W2785171078 hasRelatedWork W2025012184 @default.
- W2785171078 hasRelatedWork W2044133255 @default.
- W2785171078 hasRelatedWork W2109284489 @default.
- W2785171078 hasRelatedWork W2139680801 @default.
- W2785171078 hasRelatedWork W2158777069 @default.
- W2785171078 hasRelatedWork W2181282788 @default.
- W2785171078 hasRelatedWork W2246359456 @default.
- W2785171078 hasRelatedWork W2748113513 @default.
- W2785171078 hasRelatedWork W2766313617 @default.
- W2785171078 hasRelatedWork W2909493982 @default.
- W2785171078 hasRelatedWork W2943173276 @default.
- W2785171078 hasRelatedWork W2952165224 @default.
- W2785171078 hasRelatedWork W3099229008 @default.
- W2785171078 hasRelatedWork W3099759457 @default.
- W2785171078 hasRelatedWork W3099837933 @default.
- W2785171078 hasRelatedWork W3143022674 @default.
- W2785171078 isParatext "false" @default.
- W2785171078 isRetracted "false" @default.
- W2785171078 magId "2785171078" @default.
- W2785171078 workType "article" @default.