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• W2785318061 abstract "Abstract The successive ionic layer absorption and reaction (SILAR) method has been successfully used for the thin film preparation of metal oxides. In this work, we firstly fabricate the hybrid Bi2MoO6@Bi2Mo2O9 photoanode by a one-step SILAR method. The optimized Bi2MoO6@Bi2Mo2O9 demonstrates a photocurrent about 0.160 mA cm−2 at 1.23 V vs. RHE, which is 3.6 and 8.0 times enhancement compared with pristine Bi2MoO6 and Bi2Mo2O9 for water oxidation. The enhanced efficiencies of charge separation and oxidation kinetics by Bi2MoO6@Bi2Mo2O9 are 20.5% and 54.6% at 1.23 V vs. RHE, which is higher than Bi2Mo2O9 (9.2% and 15.4%) and Bi2MoO6 (10.7% and 29.2%). Moreover, the electron transport time of Bi2MoO6@Bi2Mo2O9 is 0.038 ms at 300 W m−2 through the controlled intensity modulated photocurrent spectrometer analysis, which is lower than Bi2Mo2O9 (0.087 ms) and Bi2MoO6 (0.052 ms). The enhanced photoelectrochemical activities of Bi2MoO6@Bi2Mo2O9 can be attributed to the matched energy band between Bi2Mo2O9 and Bi2MoO6, which could not only improve the charge separation, but also accelerate the charge migration. Therefore, our research indicates an effective technique for fabricating Bi2MoO6@Bi2Mo2O9 by one step process, and thus may provide a new idea for the preparation of other hybrid ternary metal oxides." @default.
• W2785318061 created "2018-02-23" @default.
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• W2785318061 date "2018-02-01" @default.
• W2785318061 modified "2023-10-16" @default.
• W2785318061 title "Enhanced charge separation and transfer by Bi 2 MoO 6 @Bi 2 Mo 2 O 9 compound using SILAR for photoelectrochemical water oxidation" @default.
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• W2785318061 doi "https://doi.org/10.1016/j.electacta.2018.01.090" @default.
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