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- W2785455035 abstract "Anatase TiO2 nanosheets (-ns-) with dominant exposed {001} facets were used as support to load copper, and the synthesized Cu/TiO2-ns catalysts were evaluated for CO2 hydrogenation to methanol. Under the reaction conditions, P = 3.0 MPa, T = 260 °C, V(N2):V(H2):V(CO2) = 8:69:23 and gas hourly space velocity (GHSV) = 3600 mL g−1 h−1, the methanol yield reached an appealing high value, 5.6%. Copper-loading amount, calcination temperature and reduction atmosphere have been investigated in this work, which significantly influence the particle sizes of copper and/or the defect concentration in TiO2, then leading to different catalytic performance. Characterizations of XRD, EPR, CO2-TPD and FTIR demonstrate that higher specific surface area of Cu is good for the hydrogenation of CO2 and adequate amount of Ti3+ plays important roles in CO2 activation. Both of them facilitate high turnover frequency (TOF) of methanol formation." @default.
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- W2785455035 date "2018-03-01" @default.
- W2785455035 modified "2023-10-17" @default.
- W2785455035 title "Highly efficient Cu/anatase TiO 2 {001}-nanosheets catalysts for methanol synthesis from CO 2" @default.
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- W2785455035 doi "https://doi.org/10.1016/j.jechem.2017.12.015" @default.
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