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• W2786954949 abstract "Driving by interplay between plasmonic and magnetic effects in organic composite semiconductors is a challenging task with a huge potential for practical applications. Here, we present evidence of a quantum plasmon excited in the self-assembled Co x C60 nanocomposite films with x > 15 (interval of the Co cluster coalescence) and analyse it using the optical absorption (OA) spectra. In the case of Co x C60 film with x = 16 (LF sample), the quantum plasmon generated by the Co/CoO clusters is found as the 1.5 eV-centred OA peak. This finding is supported by the establishment of four specific C60-related OA lines detected at the photon energies E p > 2.5 eV. Increase of the Co content up to x = 29 (HF sample) leads to pronounced enhancement of OA intensity in the energy range of E p > 2.5 eV and to plasmonic peak downshift of 0.2 eV with respect to the peak position in the LF spectrum. Four pairs of the OA peaks evaluated in the HF spectrum at E p > 2.5 eV reflect splitting of the C60-related lines, suggesting great change in the microscopic conditions with increasing x. Analysis of the film nanostructure and the plasmon-induced conditions allows us to propose a Rashba-like spin splitting effect that suggests valuable sources for spin polarization." @default.
• W2786954949 created "2018-02-23" @default.
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• W2786954949 date "2018-02-12" @default.
• W2786954949 modified "2023-09-28" @default.
• W2786954949 title "Quantum plasmon and Rashba-like spin splitting in self-assembled Co<i>_x</i>C₆₀composites with enhanced Co content (<i>x</i>> 15)" @default.
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• W2786954949 doi "https://doi.org/10.1088/1361-6528/aaaa7a" @default.
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