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- W2787471594 abstract "Colloidal self-assembly is a promising bottom-up route to a wide variety of three-dimensional structures, from clusters to crystals. Programming hierarchical self-assembly of colloidal building blocks, which can give rise to structures ordered at multiple levels to rival biological complexity, poses a multiscale design problem. Here we explore a generic design principle that exploits a hierarchy of interaction strengths and employ this design principle in computer simulations to demonstrate the hierarchical self-assembly of triblock patchy colloidal particles into two distinct colloidal crystals. We obtain cubic diamond and body-centered cubic crystals via distinct clusters of uniform size and shape, namely, tetrahedra and octahedra, respectively. Such a conceptual design framework has the potential to reliably encode hierarchical self-assembly of colloidal particles into a high level of sophistication. Moreover, the design framework underpins a bottom-up route to cubic diamond colloidal crystals, which have remained elusive despite being much sought after for their attractive photonic applications." @default.
- W2787471594 created "2018-02-23" @default.
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- W2787471594 date "2018-02-19" @default.
- W2787471594 modified "2023-10-17" @default.
- W2787471594 title "Programming Hierarchical Self-Assembly of Patchy Particles into Colloidal Crystals <i>via</i> Colloidal Molecules" @default.
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- W2787471594 doi "https://doi.org/10.1021/acsnano.7b07633" @default.
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- W2787471594 hasPublicationYear "2018" @default.
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