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• W2788578056 endingPage "3504" @default.
• W2788578056 startingPage "3500" @default.
• W2788578056 abstract "Many indicator displacement assays can detect biological analytes in water, but these often have reduced performance in the presence of an unavoidable component: NaCl. We report here a new self-assembled sensor, DimerDye, that uses a novel photochemical guest-sensing mechanism and that is intrinsically tolerant of cosolutes. We synthetically integrated a dye into a calixarene macrocycle, forming two new merocyanine calixarenes (MCx-1 and MCx-2). Both compounds self-assemble into nonemissive dimers in water. The addition of good guests like trimethyllysine induces a turn-on fluorescence response of MCx-1 due to simultaneous dimer dissociation and formation of an emissive host-guest complex. DimerDyes remain functional in solutions containing the various salts, metal ions, and cofactors that are needed for enzymatic reactions. MCx-1 provides a real-time, turn-on fluorescence signal in response to the lysine methyltransferase reaction of PRDM9." @default.
• W2788578056 created "2018-03-06" @default.
• W2788578056 creator A5000544946 @default.
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• W2788578056 date "2018-03-14" @default.
• W2788578056 modified "2023-10-06" @default.
• W2788578056 title "Analyte-Driven Disassembly and Turn-On Fluorescent Sensing in Competitive Biological Media." @default.
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• W2788578056 doi "https://doi.org/10.1021/jacs.7b13298" @default.
• W2788578056 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29461821" @default.
• W2788578056 hasPublicationYear "2018" @default.
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