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- W2788896664 abstract "Interfacial assemblies formed by polymeric amphiphiles at aqueous interfaces of thermotropic liquid crystals (LCs) can trigger multiscale changes in the organization of the LCs in response to recognition events. However, we have a limited understanding of the rules governing the rational design of LC-integrated polymeric amphiphiles. Herein, we report the synthesis of families of amphiphilic polymers that differ in (i) side-chain molecular structure, (ii) polymer architecture, and (iii) copolymer composition. We used this library in experiments to establish structure–property relationships relevant to the design of multifunctional polymers that can amplify and transduce biomolecular recognition events into optically detectable, macroscopic ordering transitions in LCs. We then utilized these structure–property relationships to guide the design of a peptide–polymer amphiphile (PPA) that assembles at the interface of LC droplets. Enzymatic cleavage of PPA-coated LC droplets by thermolysin directly triggered ..." @default.
- W2788896664 created "2018-03-06" @default.
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- W2788896664 date "2018-02-26" @default.
- W2788896664 modified "2023-10-18" @default.
- W2788896664 title "Design Principles for Triggerable Polymeric Amphiphiles with Mesogenic Side Chains for Multiscale Responses with Liquid Crystals" @default.
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- W2788896664 doi "https://doi.org/10.1021/acs.macromol.7b02140" @default.
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