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• W2789771987 startingPage "4902" @default.
• W2789771987 abstract "Abstract Selective decomposition of hydrous hydrazine (N 2 H 4 ⋅ H 2 O) over metal catalysts provides a promising means for onboard or portable hydrogen source applications. Studies on N 2 H 4 ⋅ H 2 O decomposition catalysts mainly focus on the effects of bulk composition and structure on their performances, instead of the surface‐composition‐dependent properties. Herein, the synthesis of an Ir‐modified Ni/ meso ‐CeO 2 catalyst is reported by using a combination of colloidal solution combustion synthesis and galvanic replacement methods. A combination of structural characterization, control experiments, and DFT calculations reveals that the Ni−Ir alloy resulting from calcination treatment exerts a profound effect on the catalytic properties. The resulting Ni@Ni−Ir/ meso ‐CeO 2 catalyst shows excellent catalytic performance towards hydrogen generation from N 2 H 4 ⋅ H 2 O, which compares favorably with the Ni−Ir bimetallic catalysts reported to date." @default.
• W2789771987 created "2018-03-29" @default.
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• W2789771987 date "2018-03-02" @default.
• W2789771987 modified "2023-10-15" @default.
• W2789771987 title "Tuning the Surface Composition of Ni/<i>meso</i>‐CeO₂ with Iridium as an Efficient Catalyst for Hydrogen Generation from Hydrous Hydrazine" @default.
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• W2789771987 doi "https://doi.org/10.1002/chem.201705923" @default.
• W2789771987 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29368412" @default.
• W2789771987 hasPublicationYear "2018" @default.
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