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• W2790097188 abstract "The development of new methods to synthesize nanometric metal catalysts has always been an important and prerequisite step in advanced catalysis. Herein, we design a stable nitrogen ligated Pt complex for the straightforward synthesis by carbonization of uniformly sized atomic and sub-nanometric Pt catalysts supported on mesoporous silica. During the carbonization of the Pt precursor into active Pt species, the nitrogen-containing ligand directed the decomposition in a controlled fashion to maintain uniform sizes of the Pt species. The nitrogen ligand had a key role to stabilize the single Pt atoms on a weak anchoring support like silica. The Pt catalysts exhibited remarkable activities in the hydrogenation of common organic functional groups with turnover frequencies higher than in previous studies. By a simple post-synthetic treatment, we could selectively remove the Pt nanoparticles to obtain a mixture of single atoms and nanoclusters, extending the applicability of the present method." @default.
• W2790097188 created "2018-03-29" @default.
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• W2790097188 date "2018-03-25" @default.
• W2790097188 modified "2023-10-03" @default.
• W2790097188 title "Designed Precursor for the Controlled Synthesis of Highly Active Atomic and Sub-nanometric Platinum Catalysts on Mesoporous Silica" @default.
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• W2790097188 doi "https://doi.org/10.1002/asia.201800125" @default.
• W2790097188 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29464882" @default.
• W2790097188 hasPublicationYear "2018" @default.
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