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• W2790457478 abstract "The coordination of CO 2 to Lewis bases is well‐known; however, its binding to Lewis acids is much less common. The ligation of CO 2 to a zinc‐substituted Wells–Dawson type polyoxometalate yielded [( n ‐C 8 H 17 ) 4 N] 8 [α 2 ‐P 2 W 17 O 61 Zn(CO 2 )], which was studied by variable temperature 1 H NMR, 13 C NMR, and 31 P NMR spectroscopy from room temperature to 201 K. The spectra were analyzed in consideration of predicted “end‐on” coordination, POM‐Zn‐O‐C‐O, and “side‐on” coordination where in addition an adjacent basic oxygen atom in the polyoxometalate binds the carbon atom of CO 2 . After adding 2,4,6‐trimethypyridine into the solution, a plausible adduct, POM‐CO 2 ‐2,4,6‐trimethypyridine, was observed." @default.
• W2790457478 created "2018-03-29" @default.
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• W2790457478 date "2018-02-05" @default.
• W2790457478 modified "2023-10-16" @default.
• W2790457478 title "Coordination of Carbon Dioxide to the Lewis Acid Site of a Zinc‐Substituted Polyoxometalate and Formation of an Adduct Using a Polyoxometalate–2,4,6‐Trimethylpyridine Frustrated Lewis Pair" @default.
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• W2790457478 doi "https://doi.org/10.1002/ejic.201701293" @default.
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