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- W2790474865 abstract "The structural complexity of mechanically interlocked molecules are very attractive to chemists owing to the challenges they present. In this article, novel mechanically interlocked molecules with a daisy-chain-containing hetero[4]rotaxane motif were efficiently synthesized. In addition, a novel integrative self-sorting strategy is demonstrated, involving an ABB-type (A for host, dibenzo-24-crown-8 (DB24C8), and B for guest, ammonium salt sites) monomer and a macrocycle host, benzo-21-crown-7 (B21C7), in which the assembled species in hydrogen-bonding-supported solvent only includes a novel daisy-chain-containing hetero[4]pseudorotaxane. The found self-sorting process involves the integrative recognition between B21C7 macrocycles and carefully designed components simultaneously containing two types of secondary ammonium ions and a host molecule, DB24C8 crown ether. The self-sorting strategy is integrative to undertake self-recognition behavior to form one single species of pseudorotaxane compared with the previous report. This self-sorting system can be used for the efficient one-pot synthesis of a daisy-chain-containing hetero[4]rotaxane in a good yield. The structure of hetero[4]rotaxane was confirmed by 1 H NMR spectroscopy and high-resolution electrospray ionization (HR-ESI) mass spectrometry." @default.
- W2790474865 created "2018-03-29" @default.
- W2790474865 creator A5019627168 @default.
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- W2790474865 creator A5046170466 @default.
- W2790474865 creator A5091577769 @default.
- W2790474865 date "2018-03-02" @default.
- W2790474865 modified "2023-09-24" @default.
- W2790474865 title "Integrative Self-Sorting: One-Pot Synthesis of a Hetero[4]rotaxane from a Daisy-Chain-Containing Hetero[4]pseudorotaxane" @default.
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- W2790474865 doi "https://doi.org/10.1002/asia.201800011" @default.
- W2790474865 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29424064" @default.
- W2790474865 hasPublicationYear "2018" @default.
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