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- W2790591808 abstract "Abstract In this work, sidechain engineering on conjugated fused‐ring acceptors for conformation locking is demonstrated as an effective molecular design strategy for high‐performance nonfullerene organic solar cells (OSCs). A novel nonfullerene acceptor (ITC6‐IC) is designed and developed by introducing long alkyl chains into the terminal electron‐donating building blocks. ITC6‐IC has achieved definite conformation with a planar structure and better solubility in common organic solvents. The weak electron‐donating hexyl upshifts the lowest unoccupied molecular orbital level of ITC6‐IC, resulting in a higher V OC in comparison to the widely used ITIC. The OSCs based on PBDB‐T:ITC6‐IC reveal a promising power conversion efficiency of 11.61% and an expected high V OC of 0.97 V. The weaker π–π stacking induced by steric hindrance affords ITC6‐IC with enhanced compatibility with polymer donors. The blend film treated with suitable thermal annealing exhibits a fibril crystallization feature with a good bicontinuous network morphology. The results indicate that the molecular design approach of ITC6‐IC can be inspirational for future development of nonfullerene acceptors for high efficiency OSCs." @default.
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- W2790591808 date "2018-01-17" @default.
- W2790591808 modified "2023-10-16" @default.
- W2790591808 title "Conformation Locking on Fused‐Ring Electron Acceptor for High‐Performance Nonfullerene Organic Solar Cells" @default.
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- W2790591808 doi "https://doi.org/10.1002/adfm.201705095" @default.
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