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- W2790993196 abstract "Porous graphitic carbon nitride polymer (p-CN-BF) with enhanced photoproduction of H2 from water was prepared by a two-step treatment process including in-situ Boron and fluorine codoping using [Emim]BF4 as dopants followed by post-calcination in air. Several techniques were employed to characterize the modified structure and elucidate the doping state of B and F. It was shown that in-situ doping method is necessary for efficient doping of heteroatoms into the molecular composition of CN. The difference of doping state of B and F was that B doping primary existing in the inside skeleton of CN, but F doping merely presents in the surface layer. The inside doped B made for the enhanced visible light absorption and the production of uniform porous structure during post-sintering process. By the synergistic effect of BF codoping and post-activation, p-CN-BF showed much enhanced photoelectron generation, transmission and separation, therefore, it performs high photocatalytic activity for H2 evolution (351 μmol h−1), which was 13 and 5 times higher than samples only modified by BF codoping (CN-BF) or post-annealing (P-CN)." @default.
- W2790993196 created "2018-03-29" @default.
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- W2790993196 date "2018-05-01" @default.
- W2790993196 modified "2023-10-18" @default.
- W2790993196 title "Post-activation of in situ B F codoped g-C3N4 for enhanced photocatalytic H2 evolution" @default.
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- W2790993196 doi "https://doi.org/10.1016/j.apsusc.2018.02.073" @default.
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