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- W2790999712 abstract "Abstract Designing new materials and structure to sustain the corrosion during operation requires better understanding on the corrosion dynamics. Observation on how the corrosion proceeds in atomic scale is thus critical. Here, using a liquid cell, we studied the real-time corrosion process of palladium@platinum (Pd@Pt) core-shell nanocubes via transmission electron microscopy (TEM). The results revealed that multiple etching pathways operatively contribute to the morphology evolution during corrosion, including galvanic etching on non-defected sites with slow kinetics and halogen-induced etching at defected sites at faster rates. Corners are the preferential corrosion sites; both etching pathways are mutually restricted during corrosion. Those insights on the interaction of nanostructures with reactive liquid environments can help better engineer the surface structure to improve the stability of electrocatalysts as well as design a new porous structure that may provide more active sites for catalysis." @default.
- W2790999712 created "2018-03-29" @default.
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- W2790999712 date "2018-03-08" @default.
- W2790999712 modified "2023-10-10" @default.
- W2790999712 title "Nanoscale kinetics of asymmetrical corrosion in core-shell nanoparticles" @default.
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- W2790999712 doi "https://doi.org/10.1038/s41467-018-03372-z" @default.
- W2790999712 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5843659" @default.
- W2790999712 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29520056" @default.
- W2790999712 hasPublicationYear "2018" @default.
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