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- W2793023275 abstract "To obtain a new low-cost catalyst that possesses well Hg0 removal activity in a broad temperature range, a series of Cu-Zrx/Cl-BC catalysts were synthesized with the application of bio-char which was activated by NH4Cl. CuO-ZrO2 as the active component largely improved Hg0 removal activity of the catalysts. The catalysts were characterized by SEM-EDX, BET, XRD, H2-TPR, XPS and FT-IR. When the CuO-ZrO2 loading value was 10%, Cu-Zr10/Cl-BC reached the best Hg0 removal efficiency (98.87%) at 120 °C and maintained over 80% until 240 °C. O2 was of benefit to Hg0 removal process especially at high temperature because it could regenerate the lattice oxygen which participated in the removal reaction. In addition, Hg0 removal was mainly determined by adsorption at low temperature and the function of oxidation increased at high temperature. The characterization results indicated that the superior performance of Cu-Zr10/Cl-BC might be ascribed to lower crystallinity, stronger redox ability and better texture properties which resulted from the interaction of CuO and ZrO2. The mechanism for Hg0 removal over Cu-Zr10/Cl-BC was also proposed on the basis of above studies." @default.
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- W2793023275 date "2018-04-01" @default.
- W2793023275 modified "2023-10-16" @default.
- W2793023275 title "A novel catalyst CuO-ZrO2 doped on Cl− activated bio-char for Hg0 removal in a broad temperature range" @default.
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- W2793023275 doi "https://doi.org/10.1016/j.fuel.2018.01.051" @default.
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