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• W2793735169 abstract "It is desirable for catalyst supports to be biodegradable, easily-modifiable, and possessing high surface area. In this work, thiolated nanocellulose sponge was prepared from hydrolytic silane condensation of cellulose nanofibrils (CNF) and used as a green support to immobilize copper cations via in situ CuII to CuI reduction and complexation. The sponge featured high porosity (90.5%) and low density (29.4 mg/cm3) with regular morphology. The sponge easily recovered 94% of its original shape in water after experiencing 80% deformation under stress of 95 kPa. When used in catalyzing hydroboration of alkynes, excellent conversion and up to 99% regioselectivity were achieved with the copper-loaded sponge. The sponge-supported catalysts worked well in the absence of additional ligands, had a broad substrate scope, and retained 93% of their activity after six catalytic cycles. This simple and scalable strategy offers an efficient route for immobilizing metal catalysts on porous supports." @default.
• W2793735169 created "2018-03-29" @default.
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• W2793735169 date "2018-07-01" @default.
• W2793735169 modified "2023-10-16" @default.
• W2793735169 title "Copper-loaded nanocellulose sponge as a sustainable catalyst for regioselective hydroboration of alkynes" @default.
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• W2793735169 doi "https://doi.org/10.1016/j.carbpol.2018.03.002" @default.
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