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• W2794330129 abstract "An inverted device structure is a more stable configuration than a regular device structure for solution-processed organic solar cells (OSCs). However, most of the solution-processed small-molecule OSCs (SM-OSCs) reported in the literature used the regular device structure, and a regular device normally exhibits a higher efficiency than an inverted device. Herein, a representative small-molecule DR3TBDTT was selected to figure out the reason for photovoltaic performance differences between regular and inverted devices. The mechanisms for a reduced open-circuit voltage (Voc) and fill factor (FF) in the inverted device were studied. The reduced Voc and FF is due to the vertical phase separation with excess [6,6]-phenyl-C71-butyric acid methyl ester near the air/blend surface, which leads to a reduction in build-in voltage and unbalanced charge transport in the inverted device. Another reason for the reduced FF is the unfavorable DR3TBDTT crystallite orientation distribution along the film thickness, which is preferential edge-on crystallites in the top layer of the blend film and the increased population of face-on crystallites in the bottom layer of the blend film. This study illustrates that the morphology plays a key role in photovoltaic performance difference between regular and inverted devices and provides useful guidelines for further optimization of the morphology of solution-processed SM-OSCs." @default.
• W2794330129 created "2018-03-29" @default.
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• W2794330129 date "2018-03-23" @default.
• W2794330129 modified "2023-10-15" @default.
• W2794330129 title "Critical Role of Vertical Phase Separation in Small-Molecule Organic Solar Cells" @default.
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• W2794330129 doi "https://doi.org/10.1021/acsami.8b00886" @default.
• W2794330129 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29569439" @default.
• W2794330129 hasPublicationYear "2018" @default.
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