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- W2796274813 abstract "A well-known limitation of hydrodynamic chromatography arises from the synergistic interaction between transverse diffusion and streamwise convection, which enhances axial dispersion through the Taylor-Aris mechanism. We show that a periodic sequence of slip/no-slip conditions at the channel walls (e.g., representing wall indentations hosting stable air pockets) can significantly reduce axial dispersion, thus enhancing separation performance. The theoretical/numerical analysis is based on a generalization of Brenner’s macrotransport approach to solute transport, here modified to account for the finite-size of the suspended particles. The most effective dispersion-taming outcome is observed when the alternating sequence of slip/no-slip conditions yields non-vanishing cross-sectional flow components. The combination of these components with the hindering interaction between the channel boundaries and the finite-sized particles gives rise to a non-trivial solution of Brenner’s problem on the unit periodic ce..." @default.
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- W2796274813 date "2018-04-01" @default.
- W2796274813 modified "2023-10-18" @default.
- W2796274813 title "Taming axial dispersion in hydrodynamic chromatography columns through wall patterning" @default.
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- W2796274813 doi "https://doi.org/10.1063/1.5022257" @default.
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