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- W2796514985 abstract "Ultrasnsitive multi-mode electron spin resonance spectroscopy in the $SrLaAlO_4$ dielectric resonator at $20~mK$ reveals ferromagnetic states of $Mn^{4+}$ impurity ion. The formation of ferromagnetic states in the $MnO_6$ complex implies to oxygen deficiency of this multi-valence $Mn^{4+}$ ion. Experiment results supports that an intricate electronic hybridization in $MnO_6$ structural instability is related to Pseudo Jahn-Teller effect. Measured dipolar hyperfine structure parameter of nucleus is $P_{scriptscriptstyleparallel} =-3.7times 10^{-4}~cm^{-1}$. Mean inverse third power of the electron distance is $langle r_q^{-3}rangle=3.325~a.u.$ assuming nuclear electric quadruple moment $Q=+0.33(1)~barn$. In such a state, giant g-factor is observed due to magneto (ferromagnetic) impedance taking in to account a two-level system on the adiabatic-potential-energy-surface. The spins exhibited parity is opposite in the interaction of highest-occupied-molecular-orbital and lowest-unoccupied-molecular-orbital coupling." @default.
- W2796514985 created "2018-04-24" @default.
- W2796514985 creator A5081431660 @default.
- W2796514985 date "2018-04-17" @default.
- W2796514985 modified "2023-09-27" @default.
- W2796514985 title "Ultrasensitive multi-mode ESR probed ferromagnetic two-level system of $Mn^{4+}$ impurity ion in the insulated $MnO_6$ complex of $SrLaAlO_4$ at $20~mK$" @default.
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