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- W2797161010 abstract "A mechanistic investigation of the acid-catalysed redox-neutral oxoarylation reaction of ynamides using electrospray ionisation mass-spectrometry (ESI-MS) and quantum chemical calculations (DFT and MP2) is presented. This study reveals the diversity of pathways and products available from an otherwise deceptively simple-looking, classical transformation: fragmentation, an unusual meta-arylation and competing α-carbonyl cation pathways are some of the alternatives unveiled by ESI-MS and mechanistic experiments. Detailed calculations explain the observed trends and rationalise the results." @default.
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- W2797161010 date "2018-01-01" @default.
- W2797161010 modified "2023-10-15" @default.
- W2797161010 title "Unusual mechanisms in Claisen rearrangements: an ionic fragmentation leading to a <i>meta</i>-selective rearrangement" @default.
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- W2797161010 doi "https://doi.org/10.1039/c7sc04736c" @default.
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