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• W2797695045 abstract "To mimic the unique properties of capsid (protein shell of a virus), we performed Brownian dynamics simulations of the self-assembly of amphiphilic truncated cone particles with anisotropic interactions. The particle shape of a truncated cone in our simulations depended on the cone angle θ, truncated height hc and particle type (A x B y and B x A y B z ). The hydrophobic A moieties and hydrophilic B moieties are responsible for attractive and repulsive interactions, respectively. By varying the particle shape, truncated cones can assemble into hollow and vesicle-like clusters with a specific cluster size N. To assemble into hollow vesicles, the truncated height hc must be below a critical value. When hc exceeds this critical value, malformation will occur. The dynamics shows that the vesicle formation occurs in three stages: initially the growth is slow, then rapid, and finally it slows down. The truncated height hc has a stronger impact on the growth kinetics than the cone angle θ or the particle type. We explored how the cluster packing depended on the cooling rate and particle number as well as discussing the relationship between the cluster geometry and the interparticle interactions. Further, we also discuss possible methods to experimentally prepare the truncated cones. The results of our work deepen our understanding of the self-assembly behavior of truncated cones and our results will aid the effective design of particle building blocks for novel nanostructures." @default.
• W2797695045 created "2018-04-24" @default.
• W2797695045 creator A5012152127 @default.
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• W2797695045 date "2018-01-01" @default.
• W2797695045 modified "2023-09-27" @default.
• W2797695045 title "Self-assembly of amphiphilic truncated cones to form hollow nanovesicles" @default.
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• W2797695045 doi "https://doi.org/10.1039/c8ra01100a" @default.
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• W2797695045 hasPublicationYear "2018" @default.
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