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• W2798989823 abstract "By selecting specific decay reactions in high-energy collisions (60 keV/amu) of hydrogen cluster ions with a helium target (utilizing event-by-event data of a recently developed multicoincidence experiment) and by deriving corresponding temperatures for these microcanonical cluster ensembles (analyzing respective fragment distributions), we are able to construct caloric curves for H+3(H2)(m) cluster ions (6<or=m<or=14). All individual curves and the mean of these curves show a backbending in the plateau region, thus constituting direct evidence for a negative microcanonical heat capacity in the liquid-to-gas transition of these finite systems." @default.
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• W2798989823 date "2002-10-11" @default.
• W2798989823 modified "2023-09-24" @default.
• W2798989823 title "Direct Experimental Evidence for a Negative Heat Capacity in the Liquid-to-Gas Phase Transition in Hydrogen Cluster Ions: Backbending of the Caloric Curve" @default.
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• W2798989823 doi "https://doi.org/10.1103/physrevlett.89.183403" @default.
• W2798989823 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/12398599" @default.
• W2798989823 hasPublicationYear "2002" @default.
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