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• W2799559329 abstract "Abstract We demonstrate, based on experimental and theoretical evidence, that the isolated [2(CH 3 CN) 2 ] 2+ complex prepared in CH 3 CN and containing a mixed‐valent {Cu 2 II,I S} core evolves towards a new [2(CH 3 CN) 3 ] 2+ species upon solvation in CH 3 CN. Unlike its type III structural analogue [2(H 2 O)(OTf)] + active toward N 2 O reduction, this new type I compound is inactive. This outcome opens new perspectives for a rational for N 2 O activation using bio‐inspired Cu/S complexes, especially on the role of the valence localization/delocalization and the Cu−Cu bond on the reactivity." @default.
• W2799559329 created "2018-05-17" @default.
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• W2799559329 date "2017-12-12" @default.
• W2799559329 modified "2023-10-18" @default.
• W2799559329 title "Valence Localization at a Bio-inspired Mixed-Valent {Cu₂ S}²⁺ Motif upon Solvation in Acetonitrile: Effect on Nitrous Oxide Reductase (N₂ Or) Activity" @default.
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• W2799559329 doi "https://doi.org/10.1002/chem.201704737" @default.
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