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• W2799740536 abstract "By performing the femtosecond-pulsed [Formula: see text]-scan experiments at a wavelength of 780[Formula: see text]nm, we report the observation of simultaneous third- and fifth-order refractive nonlinearities in the film of a side-chain azobenzene copolymer synthesized by free-radical polymerization method. Theoretically, we extend two continuous wave [Formula: see text]-scan theories suitable for the excitation of ultrafast laser pulses. First one is valid only for the situation of the sample with the pure third-order refractive nonlinearity. Second one is applicable when the sample exhibits the simultaneous third- and fifth-order refractive nonlinearities. Both [Formula: see text]-scan theories allow the precise analysis of femtosecond-pulsed [Formula: see text]-scan experimental data. Using the femtosecond time-resolved optical Kerr effect measurements, we estimate the nonlinear response time of the sample to be in the sub-picosecond regime. The physical mechanisms of the observed nonlinearity are also discussed. The high nonlinear figure of merit with ultrafast response in this polymer is desirable in nonlinear photonic devices." @default.
• W2799740536 created "2018-05-17" @default.
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• W2799740536 date "2018-03-01" @default.
• W2799740536 modified "2023-09-27" @default.
• W2799740536 title "Femtosecond-pulsed Z-scan study on third- and fifth-order refractive nonlinearities in a side-chain azobenzene copolymer film" @default.
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• W2799740536 doi "https://doi.org/10.1142/s0218863518500078" @default.
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