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• W2800285825 abstract "Abstract The ethylamine cation CH3CH2NH2+ is shown to loose CH3 accompanied by a bimodal kinetic energy release. CH3CH2NH2+ exists in two conformeric forms, which are computationally shown to be distinct minima. The barrier separating the conformers is modest compared to the energy requirement for dissociation, and the conformers are so easily interconverted that the reactions take place from a mixture of the two conformers in equilibrium. However, once a reaction begins it is conformer-specific. The reaction from one conformational origin takes place by simple cleavage along a one-dimensional reaction coordinate, whereas reaction from the other origin is by a complex reaction mechanism with a two- or possibly three-dimensional reaction coordinate. Reaction by the former mechanism is a statistical process associated with a low kinetic energy release (KER), while the latter is non-statistical giving rise to a very low KER. The experimental result is a composite signal due to the superposition of two simple Gaussians, each corresponding to their respective KER." @default.
• W2800285825 created "2018-05-17" @default.
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• W2800285825 date "2018-06-01" @default.
• W2800285825 modified "2023-09-27" @default.
• W2800285825 title "The consequences of two distinct reaction coordinates in the decomposition of the ethylamine cation conformers" @default.
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• W2800285825 doi "https://doi.org/10.1016/j.cplett.2018.04.048" @default.
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