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• W2800439889 endingPage "17860" @default.
• W2800439889 startingPage "17850" @default.
• W2800439889 abstract "High-nickel materials with core-shell structures, whose bulk is rich in nickel content and the outer shell is rich in manganese content, have been demonstrated to improve cycle stability. The high-nickel cathode material LiNi0.8Co0.1Mn0.1O2 is a very promising material for lithium-ion batteries; however, its low rate performance and especially cycle performance currently hamper further commercialization. This study presents a new synthesis method to prepare this core-shell material (LiNi0.8Co0.1Mn0.1O2@ x[Li-Mn-O], x = 0.01, 0.03, 0.06). Electrochemical data show that LiNi0.8Co0.1Mn0.1O2@ x[Li-Mn-O] ( x = 0.03, CS-0.03) exhibits the best high-rate performance, cycle stability, and thermal stability. The initial discharge capacity of the core-shell sample CS-0.03 is 118 mAh g-1, which is almost the same as the discharge capacity of pristine LiNi0.8Mn0.1Co0.1O2 (117 mAh g-1) at the rate of 10 C in the voltage range of 3.0-4.3 V. Notably the capacity decay of CS-0.03 is 18.4% after 200 cycles compared to 27% decay in capacity of the pristine sample. Furthermore, CS-0.03 exhibits better thermal cycling stability. The capacity retention of the CS-0.03 sample reached 65.1% which is over 1.3 times than that of the pristine one, whose capacity retention is 49.2% after 105 cycles (55 °C). Evidently, the core-shell structured CS-0.03 sample has excellent cycle stability and this synthesis method can be applied to other cathode materials." @default.
• W2800439889 created "2018-05-17" @default.
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• W2800439889 date "2018-05-07" @default.
• W2800439889 modified "2023-09-30" @default.
• W2800439889 title "Synthesis Method for Long Cycle Life Lithium-Ion Cathode Material: Nickel-Rich Core–Shell LiNi_0.8Co_0.1Mn_0.1O₂" @default.
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• W2800439889 doi "https://doi.org/10.1021/acsami.8b02000" @default.
• W2800439889 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/29733197" @default.
• W2800439889 hasPublicationYear "2018" @default.
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