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- W2800772309 abstract "A two-dimensional photoreactive coordination polymer (2D CP), [Zn2(Fumarate)2(H2O)2(2F-spy)4] (1) (2F-spy = 2′-fluoro-4-styrylpyridine), undergoes partial [2 + 2] cycloaddition reaction under UV light in a single-crystal-to-single-crystal manner to a three-dimensional (3D) CP [Zn2(Fumarate)2(H2O)2(2F-spy)3(rctt-2F-ppcb)0.5] (2) (where rctt-2F-ppcb = 1,3-bis(4′-pyridyl)-2,4-bis(2′-fluoro-phenyl)cyclobutane), whereas another similar photoreactive 2D CP, [Zn2(Fumarate)2(3F-spy)2] (3) (3F-spy = 3′-fluoro-4-styrylpyridine), when exposed to UV light, forms a cyclobutane ring arising from the hetero-cross-coupling of 3F-spy and fumarate, in addition to the expected cyclobutane ring, rctt-3F-ppcb (rctt-3F-ppcb = 1,3-bis(4′-pyridyl)-2,4-bis(3′-fluoro-phenyl)cyclobutane) by the [2 + 2] cycloaddition reaction of 3F-spy pairs aligned in a head-to-tail (HT) fashion. It is unusual to observe two different photoproducts in a solid-state [2 + 2] photo-cycloaddition reaction involving CPs. It is possible because the metal ions appear to support the reactions between two different types of ligands." @default.
- W2800772309 created "2018-05-17" @default.
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- W2800772309 date "2018-04-30" @default.
- W2800772309 modified "2023-09-25" @default.
- W2800772309 title "Contrast Solid-State Photoreactive Behavior of Two Two-Dimensional Zn(II) Coordination Polymers" @default.
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- W2800772309 doi "https://doi.org/10.1021/acs.cgd.8b00540" @default.
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