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• W2800974316 abstract "Abstract New fluorescent probes (m-NBBD and p-NBBD) based on BODIPY were firstly developed to detect H2O2 vapor by turn-on fluorescence in this study. The benzil and BODIPY were used as recognition group and the fluorophore, respectively, and the molecule structures of these probes were optimized. Compared to weak background fluorescence of new probes with lower quantum yield of 0.008–0.010, the corresponding products from the reaction of these probes with H2O2 successfully turn on highly green-emitting fluorescence with higher quantum yield of 0.43–0.56. m-NBBD with nitro-benzil in the meta-position of BODIPY displayed much higher fluorescence enhancement (78-fold) to H2O2 than p-NBBD with nitro-benzil in the para-position. The responding mechanism of new probes to H2O2 was investigated, and it is based on the donor-excited photo-induced electron transfer mechanism. Meanwhile, m-NBBD displayed excellent selectivity to H2O2 vapor with no interferences from nitro explosives and reactive other species. Moreover, m-NBBD showed fast response (30 s) and high sensitivity (0.94 ppb) to H2O2 vapor because of the carboxylic product of m-NBBD reacting with H2O2 to increase the adsorption capacity and the sensing efficiency. In addition, m-NBBD was successfully used for visual detection of H2O2 vapor and fluorescence imaging in living cells." @default.
• W2800974316 created "2018-05-17" @default.
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• W2800974316 date "2018-09-01" @default.
• W2800974316 modified "2023-10-16" @default.
• W2800974316 title "Development of turn-on fluorescent probes for the detection of H2O2 vapor with high selectivity and sensitivity" @default.
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• W2800974316 doi "https://doi.org/10.1016/j.snb.2018.04.140" @default.
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