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• W2801072705 abstract "Achieving up-conversion luminescence from Tb3+/Eu3+ ions was generally via a complicated energy transfer process (Yb3+ → Tm3+ → Gd3+ → Ln3+, Ln = Tb/Eu), which makes the relevant energy management rather difficult and inevitably results in impure blue luminescence of Tm3+. In this work, a facile and rational strategy is designed to integrate dual-mode luminescence from Eu3+/Tb3+ ions into NaGdF4:Yb/[email protected]4:[email protected]4:Yb/[email protected]aYF4 core-multishell nanostructure. It is found that the down-conversion energy transfer across NaGdF4@NaGdF4 interface is confined in a narrow space region of approximately 2 nm. For the up-conversion mode, the primary factor that dominates the emission intensity of Eu3+ is determined to be the molar ratio of NaGdF4:Yb/Tb component in the second shell to NaGdF4:Yb/Eu one in the core, which differs from the anisotropic filtration effect previously reported. Eventually, tunable dual-mode emission colors were achieved through simply varying the inner shell thickness of NaGdF4:Yb/Tb. The strategy of integrating dual-mode luminescence of Eu3+/Tb3+ reported here for energy management allows one to design new luminescence materials for many important applications." @default.
• W2801072705 created "2018-05-17" @default.
• W2801072705 creator A5046963841 @default.
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• W2801072705 creator A5086559201 @default.
• W2801072705 date "2018-08-01" @default.
• W2801072705 modified "2023-10-18" @default.
• W2801072705 title "Tunable green/red dual-mode luminescence via energy management in core-multishell nanoparticles" @default.
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• W2801072705 doi "https://doi.org/10.1016/j.matdes.2018.04.054" @default.
• W2801072705 hasPublicationYear "2018" @default.
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