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- W2801227988 abstract "Superamphiphilic polymers (SAPs) constructed by host–guest inclusion can self-assemble into various nanostructures in solution, which can find applications in many fields such as nanodevices, drug delivery, and template synthesis. Herein, we report the controlled self-assembly of multiple-responsive SAP based on a selective host–guest inclusion of β-cyclodextrin (β-CD) with a modified poly(ethylene glycol) (PEG) (FcC11AzoPEG) consisting of a ferrocene (Fc) end group, a C11 alkyl chain, an azobenzene (Azo) block, and a poly(ethylene glycol)methyl ether (PEG) chain. These SAPs can self-assemble into interesting nanostructures in water upon exposure to different stimuli because β-CD can be selectively included with different guests, such as Fc, Azo, and C11 alkyl chain, under different stimuli. The inclusion complex of Fc with β-CD (Fc@β-CD SAP) can form nanowire micelles in aqueous solution. The nanowire micelles can be transformed into spindle micelles with the addition of oxidant because the majority of β-CDs dissociated from the complex Fc@β-CD SAP due to a conversion of Fc to Fc+ and will preferentially include with Azo group to form another dominant inclusion complex (Azo@β-CD SAP). After UV irradiation, the spindle micelles can be further transformed into spherical micelles because most of β-CDs are excluded from the complex Azo@β-CD SAP due to a trans- to cis-Azo conversion and then form a dominant inclusion complex with C11 alkyl chains (C11@β-CD SAP). This work not only demonstrates the selective host–guest inclusion of stimuli-responsive groups modified PEG with β-CD but also provides a useful approach for construction of diverse morphologies." @default.
- W2801227988 created "2018-05-17" @default.
- W2801227988 creator A5018511746 @default.
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- W2801227988 creator A5044172075 @default.
- W2801227988 creator A5052921976 @default.
- W2801227988 creator A5086420358 @default.
- W2801227988 date "2018-04-23" @default.
- W2801227988 modified "2023-09-27" @default.
- W2801227988 title "Controlled Self-Assembly of Multiple-Responsive Superamphiphilc Polymers Based on Host–Guest Inclusions of a Modified PEG with β-Cyclodextrin" @default.
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- W2801227988 doi "https://doi.org/10.1021/acs.langmuir.8b00470" @default.
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- W2801227988 hasPublicationYear "2018" @default.
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