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- W2801383403 abstract "A fine tuning between the crystal field and the molecular field to adopt unique ground state in frustrated magnetic R2M2O7 pyrochlores structures is made by the variation of chemical pressure at R-site caused by substitution of nonmagnetic cation of M-site. Existence of larger cation at M-site increases the lattice parameter or nearest-neighbor bond distance between magnetic R-spins, and causes subtle changes to the local oxygen environment surrounding each R-ion, thereby reduces the chemical pressure at R-site which leads to a dramatic change in the crystal-field and molecular field. To investigate the effect of chemical pressure, the experimental results of powder magnetic susceptibility and isothermal magnetization of the frustrated compound Gd2Pb2O7 containing largest cation, e.g. lead (Pb), at M4+-sites were simulated and analyzed employing a D3d crystal-field (CF) and anisotropic molecular field at R-sites in the self- consistent mean-field approach. The second-ordered axial parameter B20 and total CF splitting of the ground multiplet Gd-ion in Gd2Pb2O7 are 477 cm-1 and 4.8 cm-1 respectively which are the lowest among their isomorphous counterparts, implying reduced effect of the crystal-field at Gd site in Gd2Pb2O7." @default.
- W2801383403 created "2018-05-17" @default.
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- W2801383403 date "2018-01-01" @default.
- W2801383403 modified "2023-09-27" @default.
- W2801383403 title "Study of crystal-field interaction in magnetic frustrated lead pyrochlore Gd2Pb2O7" @default.
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- W2801383403 doi "https://doi.org/10.1063/1.5033098" @default.
- W2801383403 hasPublicationYear "2018" @default.
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