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- W2801402088 abstract "We report a direct β-alkylation of ketones and aldehydes with simple alkyl bromides through a Pd-catalyzed redox-cascade strategy. The use of a Cu cocatalyst is important for improved efficiency. The reaction is redox-neutral, without the need for strong acids or bases. Both cyclic and acyclic ketones, as well as α-branched aldehydes, are suitable substrates for coupling with secondary and tertiary alkyl bromides. Concise formal synthesis of Zanapezil is achieved using this β-alkylation method." @default.
- W2801402088 created "2018-05-17" @default.
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- W2801402088 date "2018-04-30" @default.
- W2801402088 modified "2023-10-04" @default.
- W2801402088 title "Direct β-Alkylation of Ketones and Aldehydes via Pd-Catalyzed Redox Cascade" @default.
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- W2801402088 doi "https://doi.org/10.1021/jacs.8b03530" @default.
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