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• W2801608849 abstract "Structural and stoichiometric alterations in cathode materials with high intercalation voltages have been a bottleneck for next generation lithium ion batteries. Moreover, structure damage with the slightest of temperature elevation is predominant in known cathode systems. Monoclinic Li3V2(PO4)3 (LVP) with high intercalation voltage (>4.0 V) is a potential high-power cathode for lithium ion batteries owing to extraordinary stability of the phosphate anion framework. However, severe vanadium dissolution and lattice re-arrangement remains the biggest nuisance. Modification of electron conduction pathways by doping LVP lattice with Cr3+ is studied here and the efficacy of Cr3+ to stabilize the structure is understood. Vacant d-orbital sites in Cr3+ promote de-localization of electrons suppressing disproportionation and hence vanadium dissolution resulting in improved electrochemical performance for robust cycling conditions. Significant enhancement in specific capacity retention (from 26% to 84%) and improved cycle life of 400 high power cycles was observed on doping suggesting excellent performance of the cathode at high temperature (60 °C) environments." @default.
• W2801608849 created "2018-05-17" @default.
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• W2801608849 date "2018-06-01" @default.
• W2801608849 modified "2023-10-18" @default.
• W2801608849 title "Doping stabilized Li3V2(PO4)3 cathode for high voltage, temperature enduring Li-ion batteries" @default.
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• W2801608849 doi "https://doi.org/10.1016/j.jpowsour.2018.04.048" @default.
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