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• W2801789784 abstract "Ni/TiO2 catalysts with different morphologies (granular, sheet, tubular and spherical) were prepared. Hydrogen was generated from ethanol aqueous-phase reforming over Ni/TiO2 in a water-ethanol-m-chloronitrobenzene reaction system and directly applied into m-chloronitrobenzene catalytic hydrogenation. Thereby, in-situ liquid-phase hydrogenation of m-chloronitrobenzene over Ni/TiO2 without addition of molecular hydrogen was successful. Compared with granular, sheet and spherical Ni/TiO2, the nanotubular Ni/TiO2 prepared from one-step hydrothermal reaction had larger specific surface area, smaller and uniformly-distributed pore sizes and more Lewis acid sites. In-situ liquid-phase hydrogenation of m-chloronitrobenzene experiments showed the nanotubular Ni/TiO2 had the highest catalytic activity, which was ascribed to both catalyst morphology and acid sites. Firstly, the nanotubular structure endowed the catalysts with a nanoscale confinement effect and thereby high catalytic performance. Secondly, the Lewis acid sites not only accelerated water–gas shift reaction, enhancing the ethanol aqueous-phase reforming activity for hydrogen generation, but also promoted the adsorption and hydrogenation of –NO2 on the active sites of the catalysts." @default.
• W2801789784 created "2018-05-17" @default.
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• W2801789784 date "2018-04-29" @default.
• W2801789784 modified "2023-09-26" @default.
• W2801789784 title "Hydrogenation of m-Chloronitrobenzene over Different Morphologies Ni/TiO2 without Addition of Molecular Hydrogen" @default.
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• W2801789784 doi "https://doi.org/10.3390/catal8050182" @default.
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