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• W2801904562 abstract "Abstract This paper reports the direct separation of U from lanthanides (Ln) in oxide mixtures in LiCl-KCl eutectic, a method that could simplify the pyrometallurgical reprocessing of UO 2 -based spent fuels. In the melt, the mixture of UO 2 and lanthanide oxides (Ln 2 O 3 /LnO 2 ) was chloridized by AlCl 3 , and then U was selectively recovered by forming U-Al alloys through the redox reactions of U(IV)/U(III) and U(III)/Al x U. The results showed that U could be efficiently separated from lanthanides with high separation factors ( SF U/La  = 1.1 × 10 4 , SF U/Ce  = 1.6 × 10 5 , and SF U/Sm  = 2.5 × 10 4 ). X-ray diffraction analysis indicated the predominant separation products to be Al 3 U and Al 4 U, whereas the real extraction rate of U was probably affected by trace amounts of O 2− in the melt. For the first time, single-cell operation to separate U from Ln in mixed oxides is shown to be feasible by using AlCl 3 as chlorination agent followed by electrodeposition." @default.
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• W2801904562 date "2018-06-01" @default.
• W2801904562 modified "2023-09-29" @default.
• W2801904562 title "Direct separation of uranium from lanthanides (La, Nd, Ce, Sm) in oxide mixture in LiCl-KCl eutectic melt" @default.
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• W2801904562 doi "https://doi.org/10.1016/j.electacta.2018.04.140" @default.
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