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- W280202904 abstract "The high temperature equipment necessary for the investigation of oxygen reduction kinetics using microelectrodes was set up. Three types of microelectrodes were designed and fabricated. Experiments are underway to examine the microelectrodes in respect to (1) their stability in the molten carbonate environment; (2) oxygen reduction kinetics and mass transport parameters in aqueous electrolytes for comparison with similar results using other techniques; and (3) oxygen reduction kinetics and mass transport parameters in molten carbonate electrolytes. The reaction sequences for oxygen reduction in melts of various carbonate mixtures were simulated on the basis of a postulated kinetic model involving the reduction of O/sub 2//sup 2/minus// and O/sub 2/minus// ions at the electrode. Auto-catalytic reactions involving the reaction of O/sub 2//sup 2/minus// and O/sub 2/minus// species with O/sub 2/ and the neutralization reaction of O /sup 2/minus// ions by CO/sub 2/ in the melt were taken into account. Enhancement of oxygen reduction currents occurs at high rates of oxygen dissolution in the melt. Changes in the auto-catalytic reaction rates of O/sub 2//sup 2/minus// and O/sub 2/minus// affect the polarization curves significantly only in the presence of dissolved oxygen in the melt. 8 figs." @default.
- W280202904 created "2016-06-24" @default.
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- W280202904 date "1988-01-01" @default.
- W280202904 modified "2023-09-24" @default.
- W280202904 title "Oxygen electrode in molten carbonate fuel cells: Third quarterly technical progress report, February 1-April 30, 1988" @default.
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