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- W2802131851 abstract "The symmetrical configuration is attractive for electrochemical energy storage devices due to using one electrode material, but it is difficult to achieve for a rechargeable battery. Here, we propose an electrochemical activity modulation method to construct a quasi-symmetrical rechargeable battery with decoupled conversion reactions of the anionic/cationic counterparts of covalent transition metal sulfides. The modulated process contains potential window and electrolyte modulation, followed by a predesigned conversion reaction. For molybdenum disulfide (MoS2), after cathodic modulation the sulfur redox (S0 to S2−) inside MoS2 was activated as redox center of cathode, resulting in a capacity increase of one order of magnitude and high cycling stability. Meanwhile, an anodic-modulated MoS2 anode displayed high capacity due to the reversible conversion between Mox+ and Mo0. Coupling this cathode and anode, a quasi-symmetrical battery is fabricated and opens up a new direction for building high-energy electrochemical systems." @default.
- W2802131851 created "2018-05-17" @default.
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- W2802131851 date "2018-07-01" @default.
- W2802131851 modified "2023-10-16" @default.
- W2802131851 title "A Rechargeable Quasi-symmetrical MoS2 Battery" @default.
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- W2802131851 doi "https://doi.org/10.1016/j.joule.2018.04.007" @default.
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